Utilize este identificador para referenciar este registo:
https://hdl.handle.net/1822/90336
Título: | Phase matching via plasmonic modal dispersion for third harmonic generation |
Autor(es): | Wang, Zhe Wang, Zhe Kalathingal, Vijith Ho, Yi Wei Hoang, Thanh Xuan Chu, Hong-Son Guo, Yongxin Viana-Gomes, Jose Carlos Eda, Goki Nijhuis, Christian A. |
Palavras-chave: | Plasmonics Third Harmonic Generation Phase Matching via Modal Dispersion modal phase matching nonlinear polymers plasmonic modes plasmonic waveguides two-wire transmission lines |
Data: | 25-Jul-2022 |
Editora: | Wiley |
Revista: | Advanced Science |
Citação: | Z. Wang, Z. Wang, V. Kalathingal, Y. W. Ho, T. X. Hoang, H.-S. Chu, Y. Guo, J. C. Viana-Gomes, G. Eda, C. A. Nijhuis, Phase Matching via Plasmonic Modal Dispersion for Third Harmonic Generation. Adv. Sci. 2022, 9, 2201180. https://doi.org/10.1002/advs.202201180 |
Resumo(s): | The overall effectiveness of nonlinear optical processes along extended nonlinear media highly depends on the fulfillment of the phase-matching condition for pump and generated fields. This is traditionally accomplished by exploiting the birefringence of nonlinear crystals requiring long interaction lengths (cm-scale). For nonbirefringent media and integrated photonic devices, modal phase matching can compensate the index mismatch. Here, the various interacting waves propagate in transverse modes with appropriate phase velocities, but they suffer from a low refractive index contrast and cm-scale interaction lengths. This work harnesses modal phase matching for third-harmonic generation (THG) in plasmonic waveguides using an organic polymer (poly[3-hexylthiophene-2,5-diyl]) as the nonlinear medium. One demonstrates experimentally an effective interaction area as small as ≈ 0.11 µm2 and the phase-matched modal dispersion results in THG efficiency as high as ≈ 10–3 W-2 within an effective length scale of ≈ 4.3 µm. THG also shows a strong correlation with the polarization of the incident laser beam, corresponding to the excitation of the antisymmetric plasmonic modes, corroborating that plasmonic modal phase matching is achieved. This large reduction in device area of orders of magnitude is interesting for various applications where space is critical (e.g., device integration or on-chip applications). |
Tipo: | Artigo |
URI: | https://hdl.handle.net/1822/90336 |
DOI: | 10.1002/advs.202201180 |
ISSN: | 2198-3844 |
e-ISSN: | 2198-3844 |
Versão da editora: | https://onlinelibrary.wiley.com/doi/10.1002/advs.202201180 |
Arbitragem científica: | yes |
Acesso: | Acesso aberto |
Aparece nas coleções: | CDF - CEP - Artigos/Papers (with refereeing) |
Ficheiros deste registo:
Ficheiro | Descrição | Tamanho | Formato | |
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Advanced Science - 2022 - Wang - Phase Matching via Plasmonic Modal Dispersion for Third Harmonic Generation.pdf | 1,66 MB | Adobe PDF | Ver/Abrir |